In 2002, she released her album No soy un ángel (I’m Not an Angel), produced by British dance producers Xenomania and the first single off the album, Vas a volverme loca, a cover version of Charlotte NIelsen’s hit “You Got Me Going Crazy”.
In 2003, Natalia released Besa mi piel (Kiss My Skin). On this album, she included 4 of her own compositions (including the first single, also called ‘Besa Mi Piel’).
Natalia has appeared on many other artists albums. In 2004, she appeared on an album by Spanish singer Tony Aguilar on a song called Vuelve. With addition to this, Natalia has appeared on American rapper AT’s album Electric Grease with the song “I Love This Game”.
Natalia took a break for a year. However, in September 2005, she made her comeback. First of all, she came first in the Spanish reality TV program Gente de Primera, where celebrities take a member of the public and transform them into pop stars. From 2010 to 2013 Natalia released six singles vía Internet: the single “Free Yourself” and “Indómita” were huge hits.